Determination of 222Rn Exhalation Rates and Health Effect Evaluation of Some Marbles and Granites Used in Van Province, Turkey: An Experimental Study


Erzen Yıldız H., Türkmenoğlu M.

Health Physics, 2026 (SCI-Expanded, Scopus) identifier identifier

  • Yayın Türü: Makale / Tam Makale
  • Basım Tarihi: 2026
  • Doi Numarası: 10.1097/hp.0000000000002129
  • Dergi Adı: Health Physics
  • Derginin Tarandığı İndeksler: Science Citation Index Expanded (SCI-EXPANDED), Scopus, BIOSIS, Chemical Abstracts Core, Environment Index
  • Anahtar Kelimeler: alpha particles, environmental, exhalation rate, radioactivity, radon
  • Van Yüzüncü Yıl Üniversitesi Adresli: Evet

Özet

Radon (222Rn) accounts for approximately 60% of natural radiation (2.4 mSv y-1) and is a well -documented concern as the primary contributor to indoor exposure. Radon itself is inert, but its decay products (218Po, 214Pb, 214Bi, and 214Po) are reactive and tend to attach to airborne aerosol particles, lodging in the respiratory tract (bronchi, bronchioles, and lungs). During the decay process, they deposit a large amount of radiation, emitting alpha particles into surrounding tissues, ultimately causing biological damage. While radon is most commonly released from soil or rocks, building materials are another potential source of indoor atmospheric pollution. The rate at which radon escapes from a solid substance or diffuses into the surrounding air is known as the solid’s “radon exhalation rate.” Accurately knowing the exhalation rate plays a crucial role in determining the radon source power in building materials and soil. This study aimed to determine the 222Rn exhalation rate and assess radiological risks in some marble and granite samples commonly used in the Van Province of Turkey. The study employed an LR-115 type II plastic film detector and a closed-box technique. After chemical etching and alpha track counting on the detector, the following parameters were calculated: CRn (radon concentration), CRa (radium concentration), EA (surface exhalation rate), EM (mass exhalation rate), Deff (annual effective dose), WLM (annual exposure), F (%) (radon emission coefficient), ARn (indoor radon concentration contribution), and ELCR (excess lifetime cancer risk). The average EA and EM values calculated for marbles were found to be 313.45 ± 10.90 mBq m-2 h-1 and 12.05 ± 0.41 mBq kg-1 h-1, respectively. The average EA and EM values for granites were found to be 313.66 ± 11.24 mBq m-2 h-1 and 12.06 ± 0.42 mBq kg-1 h-1, respectively. The highest values were obtained in sample M2. While the calculated radon concentrations were above the international limit value and the global average, radiological risk values were calculated based on data on indoor radon concentration contributions. It was determined that the use of both marble and granite samples in the construction sector did not pose any risk to human health.